A highly planar fluorinated benzothiadiazole-based conjugated polymer for high-performance organic thin-film transistors

Benjamin Nketia-Yawson, Hyo Sang Lee, Dongkyun Seo, Youngwoon Yoon, Won Tae Park, Kyungwon Kwak, Hae Jung Son, Bongsoo Kim, Yong Young Noh

Research output: Contribution to journalArticlepeer-review

147 Citations (Scopus)

Abstract

High-mobility and low-voltage-operated organic field-effect transistors (OFETs) are demonstrated by the design of a new fluorinated benzothiadiazole-based conjugated polymer with fluorinated high-k polymer dielectrics. A record-breaking high hole mobility of 9.0 cm2 V-1 s-1 for benzothiadiazole-based semiconducting polymers is achieved by the excellent planarity of the semiconducting polymer.

Original languageEnglish
Pages (from-to)3045-3052
Number of pages8
JournalAdvanced Materials
Volume27
Issue number19
DOIs
Publication statusPublished - 2015 May 20
Externally publishedYes

Keywords

  • benzothiadiazole
  • carrier mobility
  • charge transport
  • conjugated polymers
  • organic field-effect transistors
  • planar backbone

ASJC Scopus subject areas

  • Materials Science(all)
  • Mechanics of Materials
  • Mechanical Engineering

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