A reaction model for plasma coating of nanoparticles in hydrocarbon plasma

Alexander Yarin, Beniamino Rovagnati, Farzad Mashayek, Themis Matsoukas

Research output: Chapter in Book/Report/Conference proceedingConference contribution

Abstract

A detailed chemical kinetics scheme of the reactions occurring in a CH4/H2 plasma is used to model the deposition of amorphous carbon films onto submicron particle suspended in the plasma. The model includes electron-neutral, ion-neutral, and neutral-neutral reactions and solves for the radial distribution of species in the vicinity of the particle. Concentration profiles are obtained by solving simultaneously the diffusion equation for all species that deposit on the particle surface, and the Poisson equation for the charge-carrying species. To accommodate the low-pressure environment, the continuum equations are solved to within one mean-free path from the particle surface while kinetic theory is used to treat phenomena inside the vacuum sphere, i.e., at distances shorter than one mean-free path. Calculations at various plasma conditions and the results observed trends in light of available experimental data are presented. This is an abstract of a paper presented at the AIChE Annual Meeting and Fall Showcase (Cincinnati, OH 10/30/2005-11/4/2005).

Original languageEnglish
Title of host publicationAIChE Annual Meeting Conference Proceedings
Volume2005
Publication statusPublished - 2005 Dec 1
Event05AIChE: 2005 AIChE Annual Meeting and Fall Showcase - Cincinnati, OH, United States
Duration: 2005 Oct 302005 Nov 4

Other

Other05AIChE: 2005 AIChE Annual Meeting and Fall Showcase
CountryUnited States
CityCincinnati, OH
Period05/10/3005/11/4

Fingerprint

Hydrocarbons
Nanoparticles
Plasmas
Coatings
Kinetic theory
Carbon films
Amorphous carbon
Poisson equation
Amorphous films
Reaction kinetics
Deposits
Vacuum
Electrons
Ions

ASJC Scopus subject areas

  • Energy(all)

Cite this

Yarin, A., Rovagnati, B., Mashayek, F., & Matsoukas, T. (2005). A reaction model for plasma coating of nanoparticles in hydrocarbon plasma. In AIChE Annual Meeting Conference Proceedings (Vol. 2005)

A reaction model for plasma coating of nanoparticles in hydrocarbon plasma. / Yarin, Alexander; Rovagnati, Beniamino; Mashayek, Farzad; Matsoukas, Themis.

AIChE Annual Meeting Conference Proceedings. Vol. 2005 2005.

Research output: Chapter in Book/Report/Conference proceedingConference contribution

Yarin, A, Rovagnati, B, Mashayek, F & Matsoukas, T 2005, A reaction model for plasma coating of nanoparticles in hydrocarbon plasma. in AIChE Annual Meeting Conference Proceedings. vol. 2005, 05AIChE: 2005 AIChE Annual Meeting and Fall Showcase, Cincinnati, OH, United States, 05/10/30.
Yarin A, Rovagnati B, Mashayek F, Matsoukas T. A reaction model for plasma coating of nanoparticles in hydrocarbon plasma. In AIChE Annual Meeting Conference Proceedings. Vol. 2005. 2005
Yarin, Alexander ; Rovagnati, Beniamino ; Mashayek, Farzad ; Matsoukas, Themis. / A reaction model for plasma coating of nanoparticles in hydrocarbon plasma. AIChE Annual Meeting Conference Proceedings. Vol. 2005 2005.
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