All-solid-state flexible supercapacitors based on papers coated with carbon nanotubes and ionic-liquid-based gel electrolytes

Yu Jin Kang, Haegeun Chung, Chi Hwan Han, Woong Kim

Research output: Contribution to journalArticle

214 Citations (Scopus)

Abstract

All-solid-state flexible supercapacitors were fabricated using carbon nanotubes (CNTs), regular office papers, and ionic-liquid-based gel electrolytes. Flexible electrodes were made by coating CNTs on office papers by a drop-dry method. The gel electrolyte was prepared by mixing fumed silica nanopowders with ionic liquid, 1-ethyl-3-methylimidazolium bis(trifluoromethylsulfonyl)imide ([EMIM][NTf 2]). This supercapacitor showed high power and energy performance as a solid-state flexible supercapacitor. The specific capacitance of the CNT electrodes was 135Fg 1 at a current density of 2Ag 1, when considering the mass of active materials only. The maximum power and energy density of the supercapacitors were 164kWkg 1 and 41Whkg 1, respectively. Interestingly, the solid-state supercapacitor with the gel electrolyte showed comparable performance to the supercapacitors with ionic-liquid electrolyte. Moreover, the supercapacitor showed excellent stability and flexibility. The CNT/paper-and gel-based supercapacitors may hold great potential for low-cost and high-performance flexible energy storage applications.

Original languageEnglish
Article number065401
JournalNanotechnology
Volume23
Issue number6
DOIs
Publication statusPublished - 2012 Feb 17

ASJC Scopus subject areas

  • Bioengineering
  • Chemistry(all)
  • Materials Science(all)
  • Mechanics of Materials
  • Mechanical Engineering
  • Electrical and Electronic Engineering

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