Autothermal reforming of methane to syngas using co-precipitated Ni-(La2O3)1-x catalyst

Sun Hee Park, Kook Chun, Wang Lai Yoon, Sung Hyun Kim

Research output: Contribution to journalArticle

3 Citations (Scopus)

Abstract

Two different catalysts, Ni-(ZrO2) and Ni-(La2O 3)0.1-(ZrO2)0.9, were synthesized to use as catalysts in the autothermal reforming of methane. Ni-(ZrO2) catalyst without lanthanum prepared in this study has a good initial performance, but as the reactions keep progressing, the activities gradually decrease. In contrast, the activities of Ni-(La2O3) 0.1-(ZrO2)0.9 catalyst have high thermal stability and coke resistance due to the presence of La. Both methane conversion and hydrogen yield of Ni-(La2O3)0.1-(ZrO 2)0.9 in non-reduced form are better than reduced form and as good as commercial Ni-based catalyst (ICI 57-4).

Original languageEnglish
Pages (from-to)781-786
Number of pages6
JournalResearch on Chemical Intermediates
Volume34
Issue number8-9
DOIs
Publication statusPublished - 2008 Oct 1

Fingerprint

Methane
Reforming reactions
Catalysts
Lanthanum
Coke
Hydrogen
Thermodynamic stability

Keywords

  • Autothermal reforming
  • Catalyst
  • Lanthanum
  • Methane
  • Reforming

ASJC Scopus subject areas

  • Chemistry(all)

Cite this

Autothermal reforming of methane to syngas using co-precipitated Ni-(La2O3)1-x catalyst. / Park, Sun Hee; Chun, Kook; Yoon, Wang Lai; Kim, Sung Hyun.

In: Research on Chemical Intermediates, Vol. 34, No. 8-9, 01.10.2008, p. 781-786.

Research output: Contribution to journalArticle

Park, Sun Hee ; Chun, Kook ; Yoon, Wang Lai ; Kim, Sung Hyun. / Autothermal reforming of methane to syngas using co-precipitated Ni-(La2O3)1-x catalyst. In: Research on Chemical Intermediates. 2008 ; Vol. 34, No. 8-9. pp. 781-786.
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