Catalytic Nanoframes and Beyond

Taehyun Kwon, Minki Jun, Kwangyeol Lee

Research output: Contribution to journalArticlepeer-review

19 Citations (Scopus)

Abstract

The ever-increasing need for the production and expenditure of sustainable energy is a result of the astonishing rate of consumption of fossil fuels and the accompanying environmental problems. Emphasis is being directed to the generation of sustainable energy by the fuel cell and water splitting technologies. Accordingly, the development of highly efficient electrocatalysts has attracted significant interest, as the fuel cell and water splitting technologies are critically dependent on their performance. Among numerous catalyst designs under investigation, nanoframe catalysts have an intrinsically large surface area per volume and a tunable composition, which impacts the number of catalytically active sites and their intrinsic catalytic activity, respectively. Nevertheless, the structural integrity of the nanoframe during electrochemical operation is an ongoing concern. Some significant advances in the field of nanoframe catalysts have been recently accomplished, specifically geared to resolving the catalytic stability concerns and significantly boosting the intrinsic catalytic activity of the active sites. Herein, general synthetic concepts of nanoframe structures and their structure-dependent catalytic performance are summarized, along with recent notable advances in this field. A discussion on the remaining challenges and future directions, addressing the limitations of nanoframe catalysts, are also provided.

Original languageEnglish
Article number2001345
JournalAdvanced Materials
Volume32
Issue number33
DOIs
Publication statusPublished - 2020 Aug 1

Keywords

  • electrocatalysts
  • fuel cells
  • nanoframes
  • phase engineering
  • water splitting

ASJC Scopus subject areas

  • Materials Science(all)
  • Mechanics of Materials
  • Mechanical Engineering

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