Cellulosic carbon fibers with branching carbon nanotubes for enhanced electrochemical activities for bioprocessing applications

Xueyan Zhao, Xin Lu, William Tai Yin Tze, Jungbae Kim, Ping Wang

Research output: Contribution to journalArticle

7 Citations (Scopus)

Abstract

Renewable biobased carbon fibers are promising materials for large-scale electrochemical applications including chemical processing, energy storage, and biofuel cells. Their performance is, however, often limited by low activity. Herein we report that branching carbon nanotubes can enhance the activity of carbonized cellulosic fibers, such that the oxidation potential of NAD(H) was reduced to 0.55 V from 0.9 V when applied for bioprocessing. Coordinating with enzyme catalysts, such hierarchical carbon materials effectively facilitated the biotransformation of glycerol, with the total turnover number of NAD(H) over 3500 within 5 h of reaction.

Original languageEnglish
Pages (from-to)8853-8856
Number of pages4
JournalACS Applied Materials and Interfaces
Volume5
Issue number18
DOIs
Publication statusPublished - 2013 Sep 25

Keywords

  • carbon nanotubes
  • cellulosic fibers
  • cofactor regeneration
  • dihydroxyacetone
  • glycerol biotransformation
  • porous carbon electrode

ASJC Scopus subject areas

  • Materials Science(all)

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