Coherent two-dimensional optical spectroscopy

Research output: Contribution to journalArticle

540 Citations (Scopus)

Abstract

The study of coherent two-dimensional optical spectroscopy utilizing femtosecond IR-vis laser pulses have garnered great attention in the past decade since it can provide detailed and highly dense information on the molecular structure of peptides and proteins, molecular interactions and dynamics, nucleic acid structures, semiconductor dynamics chemical exchanges, population and coherence transfers in coupled multichromophore systems and many more. Such technique can be used to study chemical reaction dynamics in condensed phases including solutions, surfaces and interfaces. The spatial connectivity between any two different vibrational degrees of freedom via through-bond and through-space interactions is the key information that can be extracted from the time-resolved multidimensional spectra.

Original languageEnglish
Pages (from-to)1331-1418
Number of pages88
JournalChemical Reviews
Volume108
Issue number4
DOIs
Publication statusPublished - 2008 Apr 1

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Semiconductors
Molecular Dynamics Simulation
Molecular Structure
Nucleic Acids
Spectrum Analysis
Lasers
Peptides
Molecular interactions
Molecular structure
Population
Molecular dynamics
Chemical reactions
Laser pulses
Proteins
Semiconductor materials
Optical spectroscopy

ASJC Scopus subject areas

  • Chemistry(all)

Cite this

Coherent two-dimensional optical spectroscopy. / Cho, Minhaeng.

In: Chemical Reviews, Vol. 108, No. 4, 01.04.2008, p. 1331-1418.

Research output: Contribution to journalArticle

Cho, Minhaeng. / Coherent two-dimensional optical spectroscopy. In: Chemical Reviews. 2008 ; Vol. 108, No. 4. pp. 1331-1418.
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