Abstract
Removal of carbon monoxide from the H2-rich stream during fuel generation from hydrocarbons is a critical challenge, especially for proton exchange membrane fuel cell (PEMFC) applications. Herein, CO an initial concentration of 1.0 vol. % was successfully removed from a H2-rich stream to a residual level below 10 ppm, within the wide operating temperature range from 92 to 235 oC by utilizing a hybrid channel reactor comprising a micro-channel heat exchanger and mini-packed bed reactor. The mini-packed bed reactor contained two kinds of catalysts that promote preferential oxidation and methanation of CO in series. The hybrid micro- And mini- channel reactor (HMCR) offers not only ultimately safe operation but also easy scale-up and is adaptable to mass production of CO clean-up units.
| Original language | English |
|---|---|
| Title of host publication | 20th World Hydrogen Energy Conference, WHEC 2014 |
| Publisher | Committee of WHEC2014 |
| Pages | 1235-1240 |
| Number of pages | 6 |
| Volume | 2 |
| ISBN (Print) | 9780000000002 |
| Publication status | Published - 2014 |
| Event | 20th World Hydrogen Energy Conference, WHEC 2014 - Gwangju, Korea, Republic of Duration: 2014 Jun 15 → 2014 Jun 20 |
Other
| Other | 20th World Hydrogen Energy Conference, WHEC 2014 |
|---|---|
| Country | Korea, Republic of |
| City | Gwangju |
| Period | 14/6/15 → 14/6/20 |
Fingerprint
Keywords
- Co crean-up
- Hybrid micro- And mini-channel reactor (hmcr)
- Methanation
- Preferential oxidation of co (prox)
ASJC Scopus subject areas
- Energy Engineering and Power Technology
- Renewable Energy, Sustainability and the Environment
- Fuel Technology
Cite this
Combination of preferential CO oxidation and methanation in hybrid MCR for CO clean-up. / Lee, Chun Boo; Cho, Sung Ho; Lee, Dong Wook; Hwang, Kyung Ran; Park, Jong Soo; Kim, Sung Hyun.
20th World Hydrogen Energy Conference, WHEC 2014. Vol. 2 Committee of WHEC2014, 2014. p. 1235-1240.Research output: Chapter in Book/Report/Conference proceeding › Conference contribution
}
TY - GEN
T1 - Combination of preferential CO oxidation and methanation in hybrid MCR for CO clean-up
AU - Lee, Chun Boo
AU - Cho, Sung Ho
AU - Lee, Dong Wook
AU - Hwang, Kyung Ran
AU - Park, Jong Soo
AU - Kim, Sung Hyun
PY - 2014
Y1 - 2014
N2 - Removal of carbon monoxide from the H2-rich stream during fuel generation from hydrocarbons is a critical challenge, especially for proton exchange membrane fuel cell (PEMFC) applications. Herein, CO an initial concentration of 1.0 vol. % was successfully removed from a H2-rich stream to a residual level below 10 ppm, within the wide operating temperature range from 92 to 235 oC by utilizing a hybrid channel reactor comprising a micro-channel heat exchanger and mini-packed bed reactor. The mini-packed bed reactor contained two kinds of catalysts that promote preferential oxidation and methanation of CO in series. The hybrid micro- And mini- channel reactor (HMCR) offers not only ultimately safe operation but also easy scale-up and is adaptable to mass production of CO clean-up units.
AB - Removal of carbon monoxide from the H2-rich stream during fuel generation from hydrocarbons is a critical challenge, especially for proton exchange membrane fuel cell (PEMFC) applications. Herein, CO an initial concentration of 1.0 vol. % was successfully removed from a H2-rich stream to a residual level below 10 ppm, within the wide operating temperature range from 92 to 235 oC by utilizing a hybrid channel reactor comprising a micro-channel heat exchanger and mini-packed bed reactor. The mini-packed bed reactor contained two kinds of catalysts that promote preferential oxidation and methanation of CO in series. The hybrid micro- And mini- channel reactor (HMCR) offers not only ultimately safe operation but also easy scale-up and is adaptable to mass production of CO clean-up units.
KW - Co crean-up
KW - Hybrid micro- And mini-channel reactor (hmcr)
KW - Methanation
KW - Preferential oxidation of co (prox)
UR - http://www.scopus.com/inward/record.url?scp=84924993398&partnerID=8YFLogxK
UR - http://www.scopus.com/inward/citedby.url?scp=84924993398&partnerID=8YFLogxK
M3 - Conference contribution
AN - SCOPUS:84924993398
SN - 9780000000002
VL - 2
SP - 1235
EP - 1240
BT - 20th World Hydrogen Energy Conference, WHEC 2014
PB - Committee of WHEC2014
ER -