Correction of the Electrical and Thermal Extrinsic Effects in Thermoelectric Measurements by the Harman Method

Min Su Kang, Im Jun Roh, Yun Goo Lee, Seung Hyub Baek, Seong Keun Kim, Byeong Kwon Ju, Dow Bin Hyun, Jin Sang Kim, Beomjin Kwon

Research output: Contribution to journalArticle

7 Citations (Scopus)

Abstract

Although the Harman method evaluates the thermoelectric figure-of-merit in a rapid and simple fashion, the accuracy of this method is affected by several electrical and thermal extrinsic factors that have not been thoroughly investigated. Here, we study the relevant extrinsic effects and a correction scheme for them. A finite element model simulates the electrical potential and temperature fields of a sample, and enables the detailed analysis of electrical and thermal transport. The model predicts that the measurement strongly depends on the materials, sample geometries, and contact resistance of the electrodes. To verify the model, we measure the thermoelectric properties of Bi2-Te3 based alloys with systematically varied sample geometries and either with a point or a surface current source. By comparing the model and experimental data, we understand how the measurement conditions determine the extrinsic effects, and, furthermore, able to extract the intrinsic thermoelectric properties. A correction scheme is proposed to eliminate the associated extrinsic effects for an accurate evaluation. This work will help the Harman method be more consistent and accurate and contribute to the development of thermoelectric materials.

Original languageEnglish
Article number26507
JournalScientific Reports
Volume6
DOIs
Publication statusPublished - 2016 May 20

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temperature effects
thermoelectric materials
potential fields
geometry
contact resistance
figure of merit
temperature distribution
electrodes
evaluation

ASJC Scopus subject areas

  • General

Cite this

Correction of the Electrical and Thermal Extrinsic Effects in Thermoelectric Measurements by the Harman Method. / Kang, Min Su; Roh, Im Jun; Lee, Yun Goo; Baek, Seung Hyub; Kim, Seong Keun; Ju, Byeong Kwon; Hyun, Dow Bin; Kim, Jin Sang; Kwon, Beomjin.

In: Scientific Reports, Vol. 6, 26507, 20.05.2016.

Research output: Contribution to journalArticle

Kang, Min Su ; Roh, Im Jun ; Lee, Yun Goo ; Baek, Seung Hyub ; Kim, Seong Keun ; Ju, Byeong Kwon ; Hyun, Dow Bin ; Kim, Jin Sang ; Kwon, Beomjin. / Correction of the Electrical and Thermal Extrinsic Effects in Thermoelectric Measurements by the Harman Method. In: Scientific Reports. 2016 ; Vol. 6.
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