CO2 absorption enhancement in particles/methanol mixture

Jae Won Lee; Jung Yeul Jung; Jin Kyeong Kim; Anshik Shin; Hyojun Lim; Changdae Byun; Yong Tae Kang

CO₂ absorption enhancement in particles/methanol mixture

Jae Won Lee, Jung Yeul Jung, Jin Kyeong Kim, Anshik Shin, Hyojun Lim, Changdae Byun, Yong Tae Kang

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution

Abstract

Recently, the integrated gasification combined cycle (IGCC) has been extensively paid attention as a next-generation energy plant. The IGCC is a power plant using synthesis gases (syngas). In the IGCC, it needs to remove the acid gases such as carbon dioxide (CO₂) and hydrogen sulfide (H₂S) from the feed gas streams. In this study, the particles (i.e. zeolite or silica particles in this study) and methanol are combined into zeolite/methanol and silica/methanol mixtures to enhance the CO₂ absorption rate of the base fluid, which is methanol. The absorption experiments are performed in the bubble type absorber system equipped with mass flow controller (MFC), mass flow meter (MFM) and silica gel (which can remove water vapor in the outlet gases). The parametric analysis on the effects of the particle species and fractions on CO₂ absorption rate are carried out. The particle fractions have ranges from 0.01 to 1 wt/vol% for zeolite and from 0.01 to 1 vol% for the silica particles, respectively. The maximum CO₂ absorption enhancement compared to the pure methanol were obtained ~2.8 % at 0.05 wt/vol% of zeolite/methanol and 2.3 % at 0.05 vol% of silica/methanol mixtures, respectively. The zeolite/methanol or silica/methanol absorbents are expected to be a promising material for removing the acid gases.

Original language	English
Title of host publication	5th Asian Conference on Refrigeration and Air Conditioning, ACRA 2010 - Green Breeze from Asia
Subtitle of host publication	Frontiers of Refrigerants, Heat Transfer and System
Publisher	Japan Society of Refrigeration and Air Conditioning Engineering (JSRAE)
ISBN (Electronic)	9781634391252
Publication status	Published - 2010
Externally published	Yes
Event	5th Asian Conference on Refrigeration and Air Conditioning - Green Breeze from Asia: Frontiers of Refrigerants, Heat Transfer and System, ACRA 2010 - Tokyo, Japan Duration: 2010 Jun 7 → 2010 Jun 9

Publication series

Name	5th Asian Conference on Refrigeration and Air Conditioning, ACRA 2010 - Green Breeze from Asia: Frontiers of Refrigerants, Heat Transfer and System

Other

Other	5th Asian Conference on Refrigeration and Air Conditioning - Green Breeze from Asia: Frontiers of Refrigerants, Heat Transfer and System, ACRA 2010
Country	Japan
City	Tokyo
Period	10/6/7 → 10/6/9

Keywords

Bubble absorption
Carbone dioxide
IGCC
Methanol
Physical absorption
Rectisol
Silica
Zeolite

ASJC Scopus subject areas

Engineering(all)
Environmental Engineering

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Cite this

Lee, J. W., Jung, J. Y., Kim, J. K., Shin, A., Lim, H., Byun, C., & Kang, Y. T. (2010). CO₂ absorption enhancement in particles/methanol mixture. In 5th Asian Conference on Refrigeration and Air Conditioning, ACRA 2010 - Green Breeze from Asia: Frontiers of Refrigerants, Heat Transfer and System (5th Asian Conference on Refrigeration and Air Conditioning, ACRA 2010 - Green Breeze from Asia: Frontiers of Refrigerants, Heat Transfer and System). Japan Society of Refrigeration and Air Conditioning Engineering (JSRAE).

CO₂ absorption enhancement in particles/methanol mixture. / Lee, Jae Won; Jung, Jung Yeul; Kim, Jin Kyeong; Shin, Anshik; Lim, Hyojun; Byun, Changdae; Kang, Yong Tae.

5th Asian Conference on Refrigeration and Air Conditioning, ACRA 2010 - Green Breeze from Asia: Frontiers of Refrigerants, Heat Transfer and System. Japan Society of Refrigeration and Air Conditioning Engineering (JSRAE), 2010. (5th Asian Conference on Refrigeration and Air Conditioning, ACRA 2010 - Green Breeze from Asia: Frontiers of Refrigerants, Heat Transfer and System).

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution

Lee, JW, Jung, JY, Kim, JK, Shin, A, Lim, H, Byun, C & Kang, YT 2010, CO₂ absorption enhancement in particles/methanol mixture. in 5th Asian Conference on Refrigeration and Air Conditioning, ACRA 2010 - Green Breeze from Asia: Frontiers of Refrigerants, Heat Transfer and System. 5th Asian Conference on Refrigeration and Air Conditioning, ACRA 2010 - Green Breeze from Asia: Frontiers of Refrigerants, Heat Transfer and System, Japan Society of Refrigeration and Air Conditioning Engineering (JSRAE), 5th Asian Conference on Refrigeration and Air Conditioning - Green Breeze from Asia: Frontiers of Refrigerants, Heat Transfer and System, ACRA 2010, Tokyo, Japan, 10/6/7.

Lee JW, Jung JY, Kim JK, Shin A, Lim H, Byun C et al. CO₂ absorption enhancement in particles/methanol mixture. In 5th Asian Conference on Refrigeration and Air Conditioning, ACRA 2010 - Green Breeze from Asia: Frontiers of Refrigerants, Heat Transfer and System. Japan Society of Refrigeration and Air Conditioning Engineering (JSRAE). 2010. (5th Asian Conference on Refrigeration and Air Conditioning, ACRA 2010 - Green Breeze from Asia: Frontiers of Refrigerants, Heat Transfer and System).

Lee, Jae Won ; Jung, Jung Yeul ; Kim, Jin Kyeong ; Shin, Anshik ; Lim, Hyojun ; Byun, Changdae ; Kang, Yong Tae. / CO₂ absorption enhancement in particles/methanol mixture. 5th Asian Conference on Refrigeration and Air Conditioning, ACRA 2010 - Green Breeze from Asia: Frontiers of Refrigerants, Heat Transfer and System. Japan Society of Refrigeration and Air Conditioning Engineering (JSRAE), 2010. (5th Asian Conference on Refrigeration and Air Conditioning, ACRA 2010 - Green Breeze from Asia: Frontiers of Refrigerants, Heat Transfer and System).

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title = "CO2 absorption enhancement in particles/methanol mixture",

abstract = "Recently, the integrated gasification combined cycle (IGCC) has been extensively paid attention as a next-generation energy plant. The IGCC is a power plant using synthesis gases (syngas). In the IGCC, it needs to remove the acid gases such as carbon dioxide (CO2) and hydrogen sulfide (H2S) from the feed gas streams. In this study, the particles (i.e. zeolite or silica particles in this study) and methanol are combined into zeolite/methanol and silica/methanol mixtures to enhance the CO2 absorption rate of the base fluid, which is methanol. The absorption experiments are performed in the bubble type absorber system equipped with mass flow controller (MFC), mass flow meter (MFM) and silica gel (which can remove water vapor in the outlet gases). The parametric analysis on the effects of the particle species and fractions on CO2 absorption rate are carried out. The particle fractions have ranges from 0.01 to 1 wt/vol% for zeolite and from 0.01 to 1 vol% for the silica particles, respectively. The maximum CO2 absorption enhancement compared to the pure methanol were obtained ~2.8 % at 0.05 wt/vol% of zeolite/methanol and 2.3 % at 0.05 vol% of silica/methanol mixtures, respectively. The zeolite/methanol or silica/methanol absorbents are expected to be a promising material for removing the acid gases.",

keywords = "Bubble absorption, Carbone dioxide, IGCC, Methanol, Physical absorption, Rectisol, Silica, Zeolite",

author = "Lee, {Jae Won} and Jung, {Jung Yeul} and Kim, {Jin Kyeong} and Anshik Shin and Hyojun Lim and Changdae Byun and Kang, {Yong Tae}",

note = "Publisher Copyright: Copyright {\textcopyright} 2010 by the Japan Society of Refrigeration and Air Conditioning Engineering (JSRAE). Copyright: Copyright 2014 Elsevier B.V., All rights reserved.; 5th Asian Conference on Refrigeration and Air Conditioning - Green Breeze from Asia: Frontiers of Refrigerants, Heat Transfer and System, ACRA 2010 ; Conference date: 07-06-2010 Through 09-06-2010",

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AU - Lee, Jae Won

AU - Jung, Jung Yeul

AU - Kim, Jin Kyeong

AU - Shin, Anshik

AU - Lim, Hyojun

AU - Byun, Changdae

AU - Kang, Yong Tae

PY - 2010

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N2 - Recently, the integrated gasification combined cycle (IGCC) has been extensively paid attention as a next-generation energy plant. The IGCC is a power plant using synthesis gases (syngas). In the IGCC, it needs to remove the acid gases such as carbon dioxide (CO2) and hydrogen sulfide (H2S) from the feed gas streams. In this study, the particles (i.e. zeolite or silica particles in this study) and methanol are combined into zeolite/methanol and silica/methanol mixtures to enhance the CO2 absorption rate of the base fluid, which is methanol. The absorption experiments are performed in the bubble type absorber system equipped with mass flow controller (MFC), mass flow meter (MFM) and silica gel (which can remove water vapor in the outlet gases). The parametric analysis on the effects of the particle species and fractions on CO2 absorption rate are carried out. The particle fractions have ranges from 0.01 to 1 wt/vol% for zeolite and from 0.01 to 1 vol% for the silica particles, respectively. The maximum CO2 absorption enhancement compared to the pure methanol were obtained ~2.8 % at 0.05 wt/vol% of zeolite/methanol and 2.3 % at 0.05 vol% of silica/methanol mixtures, respectively. The zeolite/methanol or silica/methanol absorbents are expected to be a promising material for removing the acid gases.

AB - Recently, the integrated gasification combined cycle (IGCC) has been extensively paid attention as a next-generation energy plant. The IGCC is a power plant using synthesis gases (syngas). In the IGCC, it needs to remove the acid gases such as carbon dioxide (CO2) and hydrogen sulfide (H2S) from the feed gas streams. In this study, the particles (i.e. zeolite or silica particles in this study) and methanol are combined into zeolite/methanol and silica/methanol mixtures to enhance the CO2 absorption rate of the base fluid, which is methanol. The absorption experiments are performed in the bubble type absorber system equipped with mass flow controller (MFC), mass flow meter (MFM) and silica gel (which can remove water vapor in the outlet gases). The parametric analysis on the effects of the particle species and fractions on CO2 absorption rate are carried out. The particle fractions have ranges from 0.01 to 1 wt/vol% for zeolite and from 0.01 to 1 vol% for the silica particles, respectively. The maximum CO2 absorption enhancement compared to the pure methanol were obtained ~2.8 % at 0.05 wt/vol% of zeolite/methanol and 2.3 % at 0.05 vol% of silica/methanol mixtures, respectively. The zeolite/methanol or silica/methanol absorbents are expected to be a promising material for removing the acid gases.

KW - Bubble absorption

KW - Carbone dioxide

KW - IGCC

KW - Methanol

KW - Physical absorption

KW - Rectisol

KW - Silica

KW - Zeolite

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