Effect of Bi2O3 addition on the sintering temperature and microwave dielectric properties of Zn2 SiO4 ceramics

Jin Seong Kim; Ngoc Huan Nguyen; Myung Eun Song; Jong Bong Lim; Dong Soo Paik; Sahn Nahm; Jong Hoo Paik; Byung Hyun Choi; Soon Jae Yu

doi:10.1111/j.1744-7402.2008.02335.x

Effect of Bi₂O₃ addition on the sintering temperature and microwave dielectric properties of Zn₂ SiO₄ ceramics

Jin Seong Kim, Ngoc Huan Nguyen, Myung Eun Song, Jong Bong Lim, Dong Soo Paik, Sahn Nahm, Jong Hoo Paik, Byung Hyun Choi, Soon Jae Yu

Department of Materials Science and Engineering

Research output: Contribution to journal › Article › peer-review

16 Citations (Scopus)

Abstract

Bi₂O₃ was added to a nominal composition of Zn_1.8SiO_3.8 (ZS) ceramics to decrease their sintering temperature. When the Bi₂O₃ content was < 8.0 mol%, a porous microstructure with Bi₄ (SiO₄)₃ and SiO₂ second phases was developed in the specimen sintered at 885°C. However, when the Bi₂O₃ content exceeded 8.0 mol%, a liquid phase, which formed during sintering at temperatures below 900°C, assisted the densification of the ZS ceramics. Good microwave dielectric properties of Q × f = 12,600GHz, ε_r = 7.6, and τ_f = -22 ppm/°C were obtained from the specimen with 8.0 mol% Bi₂O₃ sintered at 885°C for 2 h.

Original language	English
Pages (from-to)	581-586
Number of pages	6
Journal	International Journal of Applied Ceramic Technology
Volume	6
Issue number	5
DOIs	https://doi.org/10.1111/j.1744-7402.2008.02335.x
Publication status	Published - 2009

ASJC Scopus subject areas

Ceramics and Composites
Condensed Matter Physics
Marketing
Materials Chemistry

Access to Document

10.1111/j.1744-7402.2008.02335.x

Cite this

@article{741b3b42e8ca49639a818ac074ff3678,

title = "Effect of Bi2O3 addition on the sintering temperature and microwave dielectric properties of Zn2 SiO4 ceramics",

abstract = "Bi2O3 was added to a nominal composition of Zn1.8SiO3.8 (ZS) ceramics to decrease their sintering temperature. When the Bi2O3 content was < 8.0 mol%, a porous microstructure with Bi4 (SiO4)3 and SiO2 second phases was developed in the specimen sintered at 885°C. However, when the Bi2O3 content exceeded 8.0 mol%, a liquid phase, which formed during sintering at temperatures below 900°C, assisted the densification of the ZS ceramics. Good microwave dielectric properties of Q × f = 12,600GHz, εr = 7.6, and τf = -22 ppm/°C were obtained from the specimen with 8.0 mol% Bi2O3 sintered at 885°C for 2 h.",

author = "Kim, {Jin Seong} and Nguyen, {Ngoc Huan} and Song, {Myung Eun} and Lim, {Jong Bong} and Paik, {Dong Soo} and Sahn Nahm and Paik, {Jong Hoo} and Choi, {Byung Hyun} and Yu, {Soon Jae}",

year = "2009",

doi = "10.1111/j.1744-7402.2008.02335.x",

language = "English",

volume = "6",

pages = "581--586",

journal = "International Journal of Applied Ceramic Technology",

issn = "1546-542X",

publisher = "Wiley-Blackwell",

number = "5",

}

TY - JOUR

T1 - Effect of Bi2O3 addition on the sintering temperature and microwave dielectric properties of Zn2 SiO4 ceramics

AU - Kim, Jin Seong

AU - Nguyen, Ngoc Huan

AU - Song, Myung Eun

AU - Lim, Jong Bong

AU - Paik, Dong Soo

AU - Nahm, Sahn

AU - Paik, Jong Hoo

AU - Choi, Byung Hyun

AU - Yu, Soon Jae

PY - 2009

Y1 - 2009

N2 - Bi2O3 was added to a nominal composition of Zn1.8SiO3.8 (ZS) ceramics to decrease their sintering temperature. When the Bi2O3 content was < 8.0 mol%, a porous microstructure with Bi4 (SiO4)3 and SiO2 second phases was developed in the specimen sintered at 885°C. However, when the Bi2O3 content exceeded 8.0 mol%, a liquid phase, which formed during sintering at temperatures below 900°C, assisted the densification of the ZS ceramics. Good microwave dielectric properties of Q × f = 12,600GHz, εr = 7.6, and τf = -22 ppm/°C were obtained from the specimen with 8.0 mol% Bi2O3 sintered at 885°C for 2 h.

AB - Bi2O3 was added to a nominal composition of Zn1.8SiO3.8 (ZS) ceramics to decrease their sintering temperature. When the Bi2O3 content was < 8.0 mol%, a porous microstructure with Bi4 (SiO4)3 and SiO2 second phases was developed in the specimen sintered at 885°C. However, when the Bi2O3 content exceeded 8.0 mol%, a liquid phase, which formed during sintering at temperatures below 900°C, assisted the densification of the ZS ceramics. Good microwave dielectric properties of Q × f = 12,600GHz, εr = 7.6, and τf = -22 ppm/°C were obtained from the specimen with 8.0 mol% Bi2O3 sintered at 885°C for 2 h.

UR - http://www.scopus.com/inward/record.url?scp=69949175492&partnerID=8YFLogxK

U2 - 10.1111/j.1744-7402.2008.02335.x

DO - 10.1111/j.1744-7402.2008.02335.x

M3 - Article

AN - SCOPUS:69949175492

SN - 1546-542X

VL - 6

SP - 581

EP - 586

JO - International Journal of Applied Ceramic Technology

JF - International Journal of Applied Ceramic Technology

IS - 5

ER -

Effect of Bi₂O₃ addition on the sintering temperature and microwave dielectric properties of Zn₂ SiO₄ ceramics

Abstract

ASJC Scopus subject areas

Access to Document

Other files and links

Fingerprint

Cite this