The effects of temperature on the nonlinear response functions associated with various two-dimensional vibrational spectroscopies (2D-VS) were discussed. Quantum mechanical expressions for the response functions were obtained in both time and frequency domains by analyzing a system-bath coupling model. 2D-VS is used for obtaining structural and dynamical information on molecules.
ASJC Scopus subject areas
- Physics and Astronomy(all)
- Physical and Theoretical Chemistry