Increasing hydrophobicity of poly(propylene) fibers by coating reduced graphene oxide and their application as depth filter media

Subramaniyan Ramasundaram, Jae Hyun Jung, Eunhyea Chung, Sung Kyu Maeng, Sang-Hyup Lee, Kyung Guen Song, Seok Won Hong

Research output: Contribution to journalArticle

12 Citations (Scopus)

Abstract

The effect of increasing the hydrophobicity of poly(propylene) (PP) fibers, the most frequently used synthetic filter materials, on depth filtration performance was investigated. Reduced graphene oxide (RGO) was employed to fabricate highly hydrophobic surfaces by a dip-coating method. The anchoring of RGO on the surface of the PP fibers was confirmed by the appearance of signals corresponding to RGO in Raman and X-ray photoelectron spectra. In addition, scanning electron microscopy images revealed the presence of wrinkled and folded RGO sheets on the PP fibers. The water contact angle increased from 108 to 125 after the first RGO coating, and it was saturated at about 135. Using kaolin as model hydrophilic particles, the depth filters with RGO-coated PP fibers showed a superior performance in terms of water flux and trans-filter pressure in comparison with those with the pristine and hydrophilic PP fibers prepared by coating functionalized GO. More importantly, particle detachment was enhanced by the hydrophobic coating during backwashing. This can be ascribed to the weakened attractive force between the RGO-coated fiber surfaces and kaolin particles due to the increase of hydrophobicity. This approach provides an effective means of enhancing the performance of synthetic fiber-based depth filters.

Original languageEnglish
Pages (from-to)179-189
Number of pages11
JournalCarbon
Volume70
DOIs
Publication statusPublished - 2014 Apr 1

Fingerprint

Graphite
Hydrophobicity
Oxides
Polypropylenes
Coatings
Fibers
Kaolin
Water
Synthetic fibers
Photoelectrons
Contact angle
Fluxes
X rays
Scanning electron microscopy
propylene

ASJC Scopus subject areas

  • Chemistry(all)

Cite this

Increasing hydrophobicity of poly(propylene) fibers by coating reduced graphene oxide and their application as depth filter media. / Ramasundaram, Subramaniyan; Jung, Jae Hyun; Chung, Eunhyea; Maeng, Sung Kyu; Lee, Sang-Hyup; Song, Kyung Guen; Hong, Seok Won.

In: Carbon, Vol. 70, 01.04.2014, p. 179-189.

Research output: Contribution to journalArticle

Ramasundaram, Subramaniyan ; Jung, Jae Hyun ; Chung, Eunhyea ; Maeng, Sung Kyu ; Lee, Sang-Hyup ; Song, Kyung Guen ; Hong, Seok Won. / Increasing hydrophobicity of poly(propylene) fibers by coating reduced graphene oxide and their application as depth filter media. In: Carbon. 2014 ; Vol. 70. pp. 179-189.
@article{d0c67310dcce493499f778f44bca87f4,
title = "Increasing hydrophobicity of poly(propylene) fibers by coating reduced graphene oxide and their application as depth filter media",
abstract = "The effect of increasing the hydrophobicity of poly(propylene) (PP) fibers, the most frequently used synthetic filter materials, on depth filtration performance was investigated. Reduced graphene oxide (RGO) was employed to fabricate highly hydrophobic surfaces by a dip-coating method. The anchoring of RGO on the surface of the PP fibers was confirmed by the appearance of signals corresponding to RGO in Raman and X-ray photoelectron spectra. In addition, scanning electron microscopy images revealed the presence of wrinkled and folded RGO sheets on the PP fibers. The water contact angle increased from 108 to 125 after the first RGO coating, and it was saturated at about 135. Using kaolin as model hydrophilic particles, the depth filters with RGO-coated PP fibers showed a superior performance in terms of water flux and trans-filter pressure in comparison with those with the pristine and hydrophilic PP fibers prepared by coating functionalized GO. More importantly, particle detachment was enhanced by the hydrophobic coating during backwashing. This can be ascribed to the weakened attractive force between the RGO-coated fiber surfaces and kaolin particles due to the increase of hydrophobicity. This approach provides an effective means of enhancing the performance of synthetic fiber-based depth filters.",
author = "Subramaniyan Ramasundaram and Jung, {Jae Hyun} and Eunhyea Chung and Maeng, {Sung Kyu} and Sang-Hyup Lee and Song, {Kyung Guen} and Hong, {Seok Won}",
year = "2014",
month = "4",
day = "1",
doi = "10.1016/j.carbon.2013.12.091",
language = "English",
volume = "70",
pages = "179--189",
journal = "Carbon",
issn = "0008-6223",
publisher = "Elsevier Limited",

}

TY - JOUR

T1 - Increasing hydrophobicity of poly(propylene) fibers by coating reduced graphene oxide and their application as depth filter media

AU - Ramasundaram, Subramaniyan

AU - Jung, Jae Hyun

AU - Chung, Eunhyea

AU - Maeng, Sung Kyu

AU - Lee, Sang-Hyup

AU - Song, Kyung Guen

AU - Hong, Seok Won

PY - 2014/4/1

Y1 - 2014/4/1

N2 - The effect of increasing the hydrophobicity of poly(propylene) (PP) fibers, the most frequently used synthetic filter materials, on depth filtration performance was investigated. Reduced graphene oxide (RGO) was employed to fabricate highly hydrophobic surfaces by a dip-coating method. The anchoring of RGO on the surface of the PP fibers was confirmed by the appearance of signals corresponding to RGO in Raman and X-ray photoelectron spectra. In addition, scanning electron microscopy images revealed the presence of wrinkled and folded RGO sheets on the PP fibers. The water contact angle increased from 108 to 125 after the first RGO coating, and it was saturated at about 135. Using kaolin as model hydrophilic particles, the depth filters with RGO-coated PP fibers showed a superior performance in terms of water flux and trans-filter pressure in comparison with those with the pristine and hydrophilic PP fibers prepared by coating functionalized GO. More importantly, particle detachment was enhanced by the hydrophobic coating during backwashing. This can be ascribed to the weakened attractive force between the RGO-coated fiber surfaces and kaolin particles due to the increase of hydrophobicity. This approach provides an effective means of enhancing the performance of synthetic fiber-based depth filters.

AB - The effect of increasing the hydrophobicity of poly(propylene) (PP) fibers, the most frequently used synthetic filter materials, on depth filtration performance was investigated. Reduced graphene oxide (RGO) was employed to fabricate highly hydrophobic surfaces by a dip-coating method. The anchoring of RGO on the surface of the PP fibers was confirmed by the appearance of signals corresponding to RGO in Raman and X-ray photoelectron spectra. In addition, scanning electron microscopy images revealed the presence of wrinkled and folded RGO sheets on the PP fibers. The water contact angle increased from 108 to 125 after the first RGO coating, and it was saturated at about 135. Using kaolin as model hydrophilic particles, the depth filters with RGO-coated PP fibers showed a superior performance in terms of water flux and trans-filter pressure in comparison with those with the pristine and hydrophilic PP fibers prepared by coating functionalized GO. More importantly, particle detachment was enhanced by the hydrophobic coating during backwashing. This can be ascribed to the weakened attractive force between the RGO-coated fiber surfaces and kaolin particles due to the increase of hydrophobicity. This approach provides an effective means of enhancing the performance of synthetic fiber-based depth filters.

UR - http://www.scopus.com/inward/record.url?scp=84895060810&partnerID=8YFLogxK

UR - http://www.scopus.com/inward/citedby.url?scp=84895060810&partnerID=8YFLogxK

U2 - 10.1016/j.carbon.2013.12.091

DO - 10.1016/j.carbon.2013.12.091

M3 - Article

AN - SCOPUS:84895060810

VL - 70

SP - 179

EP - 189

JO - Carbon

JF - Carbon

SN - 0008-6223

ER -