Magnetic and neutron diffraction studies of long-range ferromagnetic order in monolayered manganites

Chang Seop Hong, Wan Seop Kim, Nam Hwi Hur, Yong Nam Choi

Research output: Contribution to journalArticle

2 Citations (Scopus)

Abstract

The structural, magnetic, and electrical properties of single crystals of Ru-doped monolayered manganites La0.5Sr1.5Mn 1-xRuxO4 (0≤x≤0.5) were investigated by neutron-diffraction, magnetization, and transport measurements. With increasing Ru content, the magnetic ground state changed from the parent antiferromagnetic (AFM) to the spin-glass to the ferromagnetic (FM) phase. The temperature-dependent neutron-diffraction measurements at x=0.35 clearly revealed long-range FM order in the monolayered manganite, which was confirmed by bulk magnetometry. The uniaxial magnetic anisotropy, in which the Ru spins are aligned along the c axis, was also observed in the compounds. This unique magnetic behavior might be ascribed to the magnetic anisotropy of the Ru ions stabilized under the structural distortion, as well as the FM ordering of Mn spins induced by AFM coupling among Mn/Ru pairs. The magnetoresistance of the Ru-doped system, which exhibits conduction confinement within a layer, diminishes with increasing Ru doping because of an increase in the proportion of FM domains at the expense of the magnetic glassy state.

Original languageEnglish
Article number064425
Pages (from-to)644251-644258
Number of pages8
JournalPhysical Review B - Condensed Matter and Materials Physics
Volume68
Issue number6
Publication statusPublished - 2003 Aug 1
Externally publishedYes

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Manganites
Magnetic anisotropy
Neutron diffraction
neutron diffraction
anisotropy
Spin glass
Magnetoresistance
diffraction
spin glass
Ground state
magnetic measurement
Structural properties
Magnetization
Magnetic properties
proportion
Electric properties
electrical properties
Doping (additives)
Single crystals
Ions

ASJC Scopus subject areas

  • Condensed Matter Physics

Cite this

Magnetic and neutron diffraction studies of long-range ferromagnetic order in monolayered manganites. / Hong, Chang Seop; Kim, Wan Seop; Hur, Nam Hwi; Choi, Yong Nam.

In: Physical Review B - Condensed Matter and Materials Physics, Vol. 68, No. 6, 064425, 01.08.2003, p. 644251-644258.

Research output: Contribution to journalArticle

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