Abstract
In the present research, the degradation of an emerging pharmaceutical micro-pollutant, Ibuprofen (IBP) by using Pd@Fe3O4 and a hybrid sono-electrolytical (US/EC) treatment system has been demonstrated for the first time. The magnetically separable nanocomposite, Pd@Fe3O4 catalyst was synthesized following co-precipitation method to enhance the efficiency of US/EC system. The synthesized catalyst showed a strong reusable property even after applying for five times and in all the five cases, 100% degradation of IBP was maintained. It not only enhanced the IBP degradation rate, but also reduced the energy consumption of the system by ∼35%. Its strong magnetization value of 64.27 emu g-1 made it easily separable. Hence, a comprehensive knowledge on the application of combined energy based US/EC system and magnetically separable multifunctional catalysts for degradation of intractable pollutants like Ibuprofen was achieved, assuring that US/EC can be an effective option for IBP treatment.
| Original language | English |
|---|---|
| Pages (from-to) | 262-272 |
| Number of pages | 11 |
| Journal | Ultrasonics Sonochemistry |
| Volume | 34 |
| DOIs | |
| Publication status | Published - 2017 Jan 1 |
Fingerprint
Keywords
- Electrolysis
- Hybrid
- Ibuprofen
- Pd@FeO
- Sonolysis
ASJC Scopus subject areas
- Chemical Engineering (miscellaneous)
- Acoustics and Ultrasonics
- Radiology Nuclear Medicine and imaging
Cite this
Magnetic Pd@Fe3O4 composite nanostructure as recoverable catalyst for sonoelectrohybrid degradation of Ibuprofen. / Thokchom, Binota; Qiu, Pengpeng; Cui, Mingcan; Park, Beomguk; Pandit, Aniruddha B.; Khim, Jeehyeong.
In: Ultrasonics Sonochemistry, Vol. 34, 01.01.2017, p. 262-272.Research output: Contribution to journal › Article
}
TY - JOUR
T1 - Magnetic Pd@Fe3O4 composite nanostructure as recoverable catalyst for sonoelectrohybrid degradation of Ibuprofen
AU - Thokchom, Binota
AU - Qiu, Pengpeng
AU - Cui, Mingcan
AU - Park, Beomguk
AU - Pandit, Aniruddha B.
AU - Khim, Jeehyeong
PY - 2017/1/1
Y1 - 2017/1/1
N2 - In the present research, the degradation of an emerging pharmaceutical micro-pollutant, Ibuprofen (IBP) by using Pd@Fe3O4 and a hybrid sono-electrolytical (US/EC) treatment system has been demonstrated for the first time. The magnetically separable nanocomposite, Pd@Fe3O4 catalyst was synthesized following co-precipitation method to enhance the efficiency of US/EC system. The synthesized catalyst showed a strong reusable property even after applying for five times and in all the five cases, 100% degradation of IBP was maintained. It not only enhanced the IBP degradation rate, but also reduced the energy consumption of the system by ∼35%. Its strong magnetization value of 64.27 emu g-1 made it easily separable. Hence, a comprehensive knowledge on the application of combined energy based US/EC system and magnetically separable multifunctional catalysts for degradation of intractable pollutants like Ibuprofen was achieved, assuring that US/EC can be an effective option for IBP treatment.
AB - In the present research, the degradation of an emerging pharmaceutical micro-pollutant, Ibuprofen (IBP) by using Pd@Fe3O4 and a hybrid sono-electrolytical (US/EC) treatment system has been demonstrated for the first time. The magnetically separable nanocomposite, Pd@Fe3O4 catalyst was synthesized following co-precipitation method to enhance the efficiency of US/EC system. The synthesized catalyst showed a strong reusable property even after applying for five times and in all the five cases, 100% degradation of IBP was maintained. It not only enhanced the IBP degradation rate, but also reduced the energy consumption of the system by ∼35%. Its strong magnetization value of 64.27 emu g-1 made it easily separable. Hence, a comprehensive knowledge on the application of combined energy based US/EC system and magnetically separable multifunctional catalysts for degradation of intractable pollutants like Ibuprofen was achieved, assuring that US/EC can be an effective option for IBP treatment.
KW - Electrolysis
KW - Hybrid
KW - Ibuprofen
KW - Pd@FeO
KW - Sonolysis
UR - http://www.scopus.com/inward/record.url?scp=84974602093&partnerID=8YFLogxK
UR - http://www.scopus.com/inward/citedby.url?scp=84974602093&partnerID=8YFLogxK
U2 - 10.1016/j.ultsonch.2016.05.030
DO - 10.1016/j.ultsonch.2016.05.030
M3 - Article
C2 - 27773244
AN - SCOPUS:84974602093
VL - 34
SP - 262
EP - 272
JO - Ultrasonics Sonochemistry
JF - Ultrasonics Sonochemistry
SN - 1350-4177
ER -