TY - CHAP
T1 - Nonlinear spectroscopy of chromophores in condensed phases with multiple frequency combs
AU - Kim, Jun Woo
AU - Cho, Minhaeng
N1 - Funding Information:
This work was supported by IBS-R023-D1.
Publisher Copyright:
© 2019, Springer Nature Singapore Pte Ltd.
Copyright:
Copyright 2019 Elsevier B.V., All rights reserved.
PY - 2019
Y1 - 2019
N2 - Coherent multidimensional spectroscopy involves more than one pulsed field-matter interaction, which creates nonlinear polarization in an optical sample and generates phase-matched coherently emitted electromagnetic fields under detection. To maintain the coherence of the involved electromagnetic fields, each single laser pulse is split into multiple pulses that remain in a fixed relative phase within their coherence lengths. However, multi-comb nonlinear spectroscopy breaks this conventional paradigm in that two or more frequency-comb lasers, which are phase stabilized and locked with one another, are used to create nonlinear polarization in the optical sample. In this chapter, nonlinear spectroscopic research utilizing two frequency combs is summarized and explained in terms of the nonlinear response function. In addition to a review of linear and nonlinear dual frequency-comb spectroscopy theory and applications, we discuss the future possibilities for the development of multi-comb nonlinear spectroscopy.
AB - Coherent multidimensional spectroscopy involves more than one pulsed field-matter interaction, which creates nonlinear polarization in an optical sample and generates phase-matched coherently emitted electromagnetic fields under detection. To maintain the coherence of the involved electromagnetic fields, each single laser pulse is split into multiple pulses that remain in a fixed relative phase within their coherence lengths. However, multi-comb nonlinear spectroscopy breaks this conventional paradigm in that two or more frequency-comb lasers, which are phase stabilized and locked with one another, are used to create nonlinear polarization in the optical sample. In this chapter, nonlinear spectroscopic research utilizing two frequency combs is summarized and explained in terms of the nonlinear response function. In addition to a review of linear and nonlinear dual frequency-comb spectroscopy theory and applications, we discuss the future possibilities for the development of multi-comb nonlinear spectroscopy.
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U2 - 10.1007/978-981-13-9753-0_16
DO - 10.1007/978-981-13-9753-0_16
M3 - Chapter
AN - SCOPUS:85070619371
T3 - Springer Series in Optical Sciences
SP - 355
EP - 379
BT - Springer Series in Optical Sciences
PB - Springer Verlag
ER -