Nonlinear spectroscopy of chromophores in condensed phases with multiple frequency combs

Jun Woo Kim, Minhaeng Cho

Research output: Chapter in Book/Report/Conference proceedingChapter

Abstract

Coherent multidimensional spectroscopy involves more than one pulsed field-matter interaction, which creates nonlinear polarization in an optical sample and generates phase-matched coherently emitted electromagnetic fields under detection. To maintain the coherence of the involved electromagnetic fields, each single laser pulse is split into multiple pulses that remain in a fixed relative phase within their coherence lengths. However, multi-comb nonlinear spectroscopy breaks this conventional paradigm in that two or more frequency-comb lasers, which are phase stabilized and locked with one another, are used to create nonlinear polarization in the optical sample. In this chapter, nonlinear spectroscopic research utilizing two frequency combs is summarized and explained in terms of the nonlinear response function. In addition to a review of linear and nonlinear dual frequency-comb spectroscopy theory and applications, we discuss the future possibilities for the development of multi-comb nonlinear spectroscopy.

Original languageEnglish
Title of host publicationSpringer Series in Optical Sciences
PublisherSpringer Verlag
Pages355-379
Number of pages25
DOIs
Publication statusPublished - 2019 Jan 1

Publication series

NameSpringer Series in Optical Sciences
Volume226
ISSN (Print)0342-4111
ISSN (Electronic)1556-1534

ASJC Scopus subject areas

  • Electronic, Optical and Magnetic Materials

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  • Cite this

    Kim, J. W., & Cho, M. (2019). Nonlinear spectroscopy of chromophores in condensed phases with multiple frequency combs. In Springer Series in Optical Sciences (pp. 355-379). (Springer Series in Optical Sciences; Vol. 226). Springer Verlag. https://doi.org/10.1007/978-981-13-9753-0_16