Abstract
Coherent multidimensional spectroscopy involves more than one pulsed field-matter interaction, which creates nonlinear polarization in an optical sample and generates phase-matched coherently emitted electromagnetic fields under detection. To maintain the coherence of the involved electromagnetic fields, each single laser pulse is split into multiple pulses that remain in a fixed relative phase within their coherence lengths. However, multi-comb nonlinear spectroscopy breaks this conventional paradigm in that two or more frequency-comb lasers, which are phase stabilized and locked with one another, are used to create nonlinear polarization in the optical sample. In this chapter, nonlinear spectroscopic research utilizing two frequency combs is summarized and explained in terms of the nonlinear response function. In addition to a review of linear and nonlinear dual frequency-comb spectroscopy theory and applications, we discuss the future possibilities for the development of multi-comb nonlinear spectroscopy.
| Original language | English |
|---|---|
| Title of host publication | Springer Series in Optical Sciences |
| Publisher | Springer Verlag |
| Pages | 355-379 |
| Number of pages | 25 |
| DOIs | |
| Publication status | Published - 2019 Jan 1 |
Publication series
| Name | Springer Series in Optical Sciences |
|---|---|
| Volume | 226 |
| ISSN (Print) | 0342-4111 |
| ISSN (Electronic) | 1556-1534 |
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ASJC Scopus subject areas
- Electronic, Optical and Magnetic Materials
Cite this
Nonlinear spectroscopy of chromophores in condensed phases with multiple frequency combs. / Kim, Jun Woo; Cho, Minhaeng.
Springer Series in Optical Sciences. Springer Verlag, 2019. p. 355-379 (Springer Series in Optical Sciences; Vol. 226).Research output: Chapter in Book/Report/Conference proceeding › Chapter
}
TY - CHAP
T1 - Nonlinear spectroscopy of chromophores in condensed phases with multiple frequency combs
AU - Kim, Jun Woo
AU - Cho, Minhaeng
PY - 2019/1/1
Y1 - 2019/1/1
N2 - Coherent multidimensional spectroscopy involves more than one pulsed field-matter interaction, which creates nonlinear polarization in an optical sample and generates phase-matched coherently emitted electromagnetic fields under detection. To maintain the coherence of the involved electromagnetic fields, each single laser pulse is split into multiple pulses that remain in a fixed relative phase within their coherence lengths. However, multi-comb nonlinear spectroscopy breaks this conventional paradigm in that two or more frequency-comb lasers, which are phase stabilized and locked with one another, are used to create nonlinear polarization in the optical sample. In this chapter, nonlinear spectroscopic research utilizing two frequency combs is summarized and explained in terms of the nonlinear response function. In addition to a review of linear and nonlinear dual frequency-comb spectroscopy theory and applications, we discuss the future possibilities for the development of multi-comb nonlinear spectroscopy.
AB - Coherent multidimensional spectroscopy involves more than one pulsed field-matter interaction, which creates nonlinear polarization in an optical sample and generates phase-matched coherently emitted electromagnetic fields under detection. To maintain the coherence of the involved electromagnetic fields, each single laser pulse is split into multiple pulses that remain in a fixed relative phase within their coherence lengths. However, multi-comb nonlinear spectroscopy breaks this conventional paradigm in that two or more frequency-comb lasers, which are phase stabilized and locked with one another, are used to create nonlinear polarization in the optical sample. In this chapter, nonlinear spectroscopic research utilizing two frequency combs is summarized and explained in terms of the nonlinear response function. In addition to a review of linear and nonlinear dual frequency-comb spectroscopy theory and applications, we discuss the future possibilities for the development of multi-comb nonlinear spectroscopy.
UR - http://www.scopus.com/inward/record.url?scp=85070619371&partnerID=8YFLogxK
UR - http://www.scopus.com/inward/citedby.url?scp=85070619371&partnerID=8YFLogxK
U2 - 10.1007/978-981-13-9753-0_16
DO - 10.1007/978-981-13-9753-0_16
M3 - Chapter
AN - SCOPUS:85070619371
T3 - Springer Series in Optical Sciences
SP - 355
EP - 379
BT - Springer Series in Optical Sciences
PB - Springer Verlag
ER -