Nuclear magnetic resonance study of the hydrogen-mediated ferromagnetic coupling in Mn-doped ZnO

Jun Kue Park; Kyu Won Lee; Cheol Eui Lee

doi:10.1016/j.ssc.2013.04.028

Nuclear magnetic resonance study of the hydrogen-mediated ferromagnetic coupling in Mn-doped ZnO

Jun Kue Park, Kyu Won Lee, Cheol Eui Lee

Department of Physics

Research output: Contribution to journal › Article › peer-review

1 Citation (Scopus)

Abstract

In our ¹H nuclear magnetic resonance study of a high-concentration Mn-doped ZnO system, the Mn-ion impurity and the proton dipole-dipole relaxation contributions were well resolved. In particular, a change at 290 K in the magnetic susceptibility showing a weakening of the ferromagnetic exchange interaction was accompanied by that in the impurity relaxation mechanism and by activation of the high-temperature hopping motion of interstitial H. Thus, a unique opportunity has been provided to elucidate the role of hydrogen in the ferromagnetic coupling in the Mn-doped ZnO systems.

Original language	English
Pages (from-to)	16-18
Number of pages	3
Journal	Solid State Communications
Volume	166
DOIs	https://doi.org/10.1016/j.ssc.2013.04.028
Publication status	Published - 2013

Keywords

A. Mn-doped ZnO
B. Sol-gel processing
D. Hydrogen-mediated ferromagnetic coupling
E. Nuclear magnetic relaxation

ASJC Scopus subject areas

Chemistry(all)
Condensed Matter Physics
Materials Chemistry

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10.1016/j.ssc.2013.04.028

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title = "Nuclear magnetic resonance study of the hydrogen-mediated ferromagnetic coupling in Mn-doped ZnO",

abstract = "In our 1H nuclear magnetic resonance study of a high-concentration Mn-doped ZnO system, the Mn-ion impurity and the proton dipole-dipole relaxation contributions were well resolved. In particular, a change at 290 K in the magnetic susceptibility showing a weakening of the ferromagnetic exchange interaction was accompanied by that in the impurity relaxation mechanism and by activation of the high-temperature hopping motion of interstitial H. Thus, a unique opportunity has been provided to elucidate the role of hydrogen in the ferromagnetic coupling in the Mn-doped ZnO systems.",

keywords = "A. Mn-doped ZnO, B. Sol-gel processing, D. Hydrogen-mediated ferromagnetic coupling, E. Nuclear magnetic relaxation",

author = "Park, {Jun Kue} and Lee, {Kyu Won} and Lee, {Cheol Eui}",

year = "2013",

doi = "10.1016/j.ssc.2013.04.028",

language = "English",

volume = "166",

pages = "16--18",

journal = "Solid State Communications",

issn = "0038-1098",

publisher = "Elsevier Limited",

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TY - JOUR

T1 - Nuclear magnetic resonance study of the hydrogen-mediated ferromagnetic coupling in Mn-doped ZnO

AU - Park, Jun Kue

AU - Lee, Kyu Won

AU - Lee, Cheol Eui

PY - 2013

Y1 - 2013

N2 - In our 1H nuclear magnetic resonance study of a high-concentration Mn-doped ZnO system, the Mn-ion impurity and the proton dipole-dipole relaxation contributions were well resolved. In particular, a change at 290 K in the magnetic susceptibility showing a weakening of the ferromagnetic exchange interaction was accompanied by that in the impurity relaxation mechanism and by activation of the high-temperature hopping motion of interstitial H. Thus, a unique opportunity has been provided to elucidate the role of hydrogen in the ferromagnetic coupling in the Mn-doped ZnO systems.

AB - In our 1H nuclear magnetic resonance study of a high-concentration Mn-doped ZnO system, the Mn-ion impurity and the proton dipole-dipole relaxation contributions were well resolved. In particular, a change at 290 K in the magnetic susceptibility showing a weakening of the ferromagnetic exchange interaction was accompanied by that in the impurity relaxation mechanism and by activation of the high-temperature hopping motion of interstitial H. Thus, a unique opportunity has been provided to elucidate the role of hydrogen in the ferromagnetic coupling in the Mn-doped ZnO systems.

KW - A. Mn-doped ZnO

KW - B. Sol-gel processing

KW - D. Hydrogen-mediated ferromagnetic coupling

KW - E. Nuclear magnetic relaxation

UR - http://www.scopus.com/inward/record.url?scp=84885400275&partnerID=8YFLogxK

UR - http://www.scopus.com/inward/citedby.url?scp=84885400275&partnerID=8YFLogxK

U2 - 10.1016/j.ssc.2013.04.028

DO - 10.1016/j.ssc.2013.04.028

M3 - Article

AN - SCOPUS:84885400275

VL - 166

SP - 16

EP - 18

JO - Solid State Communications

JF - Solid State Communications

SN - 0038-1098

ER -

Nuclear magnetic resonance study of the hydrogen-mediated ferromagnetic coupling in Mn-doped ZnO

Abstract

Keywords

ASJC Scopus subject areas

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