Paper-Like, Thin, Foldable, and Self-Healable Electronics Based on PVA/CNC Nanocomposite Film

Jung Wook Kim, Heun Park, Geumbee Lee, Yu Ra Jeong, Soo Yeong Hong, Kayeon Keum, Junyeong Yoon, Min Su Kim, Jeong Sook Ha

Research output: Contribution to journalArticle

2 Citations (Scopus)

Abstract

The facile fabrication of thin and foldable self-healing electronics on a poly(vinyl alcohol)/cellulose nanocrystal (PVA/CNC) composite film is reported. The self-healing property of the PVA/CNC nanocomposite film can be activated by spraying water on the film surface, via dynamic formation of hydrogen bonding. The self-healing efficiency of PVA/CNC is influenced by the content of CNC in the film, pH of the spraying solution, and the temperature. Via vacuum filtration and pattern transfer techniques, both a supercapacitor and a temperature sensor are fabricated on the same PVA/CNC film using gold nanosheet (AuNS) and polyaniline/multiwalled nanotube (PANI/MWCNT) electrodes. The fabricated supercapacitor with a gel-type electrolyte exhibits a high electrochemical performance, and the thermoresistive temperature sensor shows a linear sensitivity with a fast response. Both devices exhibit superior mechanical stability and self-healing property over 100 repetitive folding and five repetitive healing cycles, respectively, retaining the device performance owing to the percolated network of the conductive materials. This work demonstrates that our paper-like thin PVA/CNC film-based self-healable devices can serve as highly durable and deformable electronics with longevity.

Original languageEnglish
Article number1905968
JournalAdvanced Functional Materials
Volume29
Issue number50
DOIs
Publication statusPublished - 2019 Dec 1

Keywords

  • foldable electronics
  • poly(vinyl alcohol)/cellulose nanocrystal nanocomposites
  • self-healing electronics
  • self-healing supercapacitors
  • thermoresistive temperature sensors

ASJC Scopus subject areas

  • Chemistry(all)
  • Materials Science(all)
  • Condensed Matter Physics

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  • Cite this

    Kim, J. W., Park, H., Lee, G., Jeong, Y. R., Hong, S. Y., Keum, K., Yoon, J., Kim, M. S., & Ha, J. S. (2019). Paper-Like, Thin, Foldable, and Self-Healable Electronics Based on PVA/CNC Nanocomposite Film. Advanced Functional Materials, 29(50), [1905968]. https://doi.org/10.1002/adfm.201905968