Partitioning of dioxins (PCDDs/Fs) in ambient air at urban residential locations

Md M. Rahman; Z. H. Shon; C. J. Ma; R. J.C. Brown; S. K. Pandey; C. G. Park; I. S. Bae; J. R. Sohn; H. O. Yoon; K. H. Kim

doi:10.1007/s13762-013-0389-7

Partitioning of dioxins (PCDDs/Fs) in ambient air at urban residential locations

Md M. Rahman, Z. H. Shon, C. J. Ma, R. J.C. Brown, S. K. Pandey, C. G. Park, I. S. Bae, J. R. Sohn, H. O. Yoon, K. H. Kim

Department of Public Health Sciences

Research output: Contribution to journal › Article › peer-review

3 Citations (Scopus)

Abstract

In this work, 17-polychlorinated dibenzo-p-dioxin/furan (PCDD/Fs) isomers were measured in ambient air at four urban sites in Seoul, Korea (from February to June 2009). The concentrations of their summed values (ΣPCDD/Fs) across all four sites ranged from 1,947 (271 WHO₀₅ TEQ) (Jong Ro) to 2,600 (349 WHO₀₅ TEQ) fg/m³ (Yang Jae) with a mean of 2,125 (± 317) fg/m³ (292 WHO₀₅ TEQ fg/m³). The sum values for the two isomer groups of ΣPCDD and ΣPCDF were 527 (30 WHO₀₅ TEQ) and 1,598 (263 WHO₀₅ TEQ) fg/m³, respectively. The concentration profile of individual species was dominated by the 2,3,4,7,8-PeCDF isomer, which contributed approximately 36 % of the ΣPCDD/Fs value. The observed temporal trends in PCDD/F concentrations were characterized by relative enhancement in the winter and spring. The relative contribution of different sources, when assessed by principal component analysis, is explained by the dominance of vehicular emissions along with coal (or gas) burning as the key source of ambient PCDD/Fs in the residential areas studied.

Original language	English
Pages (from-to)	1897-1910
Number of pages	14
Journal	International Journal of Environmental Science and Technology
Volume	11
Issue number	7
DOIs	https://doi.org/10.1007/s13762-013-0389-7
Publication status	Published - 2014 Sep 1

Keywords

Gas/particle partitioning
PCDD/Fs
Residential area
Seasonal variation

ASJC Scopus subject areas

Environmental Engineering
Environmental Chemistry
Agricultural and Biological Sciences(all)

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10.1007/s13762-013-0389-7

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Partitioning of dioxins (PCDDs/Fs) in ambient air at urban residential locations. / Rahman, Md M.; Shon, Z. H.; Ma, C. J.; Brown, R. J.C.; Pandey, S. K.; Park, C. G.; Bae, I. S.; Sohn, J. R.; Yoon, H. O.; Kim, K. H.

In: International Journal of Environmental Science and Technology, Vol. 11, No. 7, 01.09.2014, p. 1897-1910.

Research output: Contribution to journal › Article › peer-review

@article{426dc82490b549a29a3a4e127fb286ab,

title = "Partitioning of dioxins (PCDDs/Fs) in ambient air at urban residential locations",

abstract = "In this work, 17-polychlorinated dibenzo-p-dioxin/furan (PCDD/Fs) isomers were measured in ambient air at four urban sites in Seoul, Korea (from February to June 2009). The concentrations of their summed values (ΣPCDD/Fs) across all four sites ranged from 1,947 (271 WHO05 TEQ) (Jong Ro) to 2,600 (349 WHO05 TEQ) fg/m3 (Yang Jae) with a mean of 2,125 (± 317) fg/m3 (292 WHO05 TEQ fg/m3). The sum values for the two isomer groups of ΣPCDD and ΣPCDF were 527 (30 WHO05 TEQ) and 1,598 (263 WHO05 TEQ) fg/m3, respectively. The concentration profile of individual species was dominated by the 2,3,4,7,8-PeCDF isomer, which contributed approximately 36 % of the ΣPCDD/Fs value. The observed temporal trends in PCDD/F concentrations were characterized by relative enhancement in the winter and spring. The relative contribution of different sources, when assessed by principal component analysis, is explained by the dominance of vehicular emissions along with coal (or gas) burning as the key source of ambient PCDD/Fs in the residential areas studied.",

keywords = "Gas/particle partitioning, PCDD/Fs, Residential area, Seasonal variation",

author = "Rahman, {Md M.} and Shon, {Z. H.} and Ma, {C. J.} and Brown, {R. J.C.} and Pandey, {S. K.} and Park, {C. G.} and Bae, {I. S.} and Sohn, {J. R.} and Yoon, {H. O.} and Kim, {K. H.}",

note = "Funding Information: This study was supported by a National Research Foundation of Korea (NRF) grant funded by the Ministry of Education, Science and Technology (MEST) (No. 2009-0093848). The ninth author acknowledges the support made by a grant from the Korea Basic Science Institute (project No. T31603). We also acknowledge partial support made by the Human Resources Development of the Korea Institute of Energy Technology Evaluation and Planning (KETEP) grant funded by the Korea government Ministry of Knowledge Economy (No. 20094010200030). Publisher Copyright: {\textcopyright} 2013, Islamic Azad University (IAU).",

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T1 - Partitioning of dioxins (PCDDs/Fs) in ambient air at urban residential locations

AU - Rahman, Md M.

AU - Shon, Z. H.

AU - Ma, C. J.

AU - Brown, R. J.C.

AU - Pandey, S. K.

AU - Park, C. G.

AU - Bae, I. S.

AU - Sohn, J. R.

AU - Yoon, H. O.

AU - Kim, K. H.

N1 - Funding Information: This study was supported by a National Research Foundation of Korea (NRF) grant funded by the Ministry of Education, Science and Technology (MEST) (No. 2009-0093848). The ninth author acknowledges the support made by a grant from the Korea Basic Science Institute (project No. T31603). We also acknowledge partial support made by the Human Resources Development of the Korea Institute of Energy Technology Evaluation and Planning (KETEP) grant funded by the Korea government Ministry of Knowledge Economy (No. 20094010200030). Publisher Copyright: © 2013, Islamic Azad University (IAU).

PY - 2014/9/1

Y1 - 2014/9/1

N2 - In this work, 17-polychlorinated dibenzo-p-dioxin/furan (PCDD/Fs) isomers were measured in ambient air at four urban sites in Seoul, Korea (from February to June 2009). The concentrations of their summed values (ΣPCDD/Fs) across all four sites ranged from 1,947 (271 WHO05 TEQ) (Jong Ro) to 2,600 (349 WHO05 TEQ) fg/m3 (Yang Jae) with a mean of 2,125 (± 317) fg/m3 (292 WHO05 TEQ fg/m3). The sum values for the two isomer groups of ΣPCDD and ΣPCDF were 527 (30 WHO05 TEQ) and 1,598 (263 WHO05 TEQ) fg/m3, respectively. The concentration profile of individual species was dominated by the 2,3,4,7,8-PeCDF isomer, which contributed approximately 36 % of the ΣPCDD/Fs value. The observed temporal trends in PCDD/F concentrations were characterized by relative enhancement in the winter and spring. The relative contribution of different sources, when assessed by principal component analysis, is explained by the dominance of vehicular emissions along with coal (or gas) burning as the key source of ambient PCDD/Fs in the residential areas studied.

AB - In this work, 17-polychlorinated dibenzo-p-dioxin/furan (PCDD/Fs) isomers were measured in ambient air at four urban sites in Seoul, Korea (from February to June 2009). The concentrations of their summed values (ΣPCDD/Fs) across all four sites ranged from 1,947 (271 WHO05 TEQ) (Jong Ro) to 2,600 (349 WHO05 TEQ) fg/m3 (Yang Jae) with a mean of 2,125 (± 317) fg/m3 (292 WHO05 TEQ fg/m3). The sum values for the two isomer groups of ΣPCDD and ΣPCDF were 527 (30 WHO05 TEQ) and 1,598 (263 WHO05 TEQ) fg/m3, respectively. The concentration profile of individual species was dominated by the 2,3,4,7,8-PeCDF isomer, which contributed approximately 36 % of the ΣPCDD/Fs value. The observed temporal trends in PCDD/F concentrations were characterized by relative enhancement in the winter and spring. The relative contribution of different sources, when assessed by principal component analysis, is explained by the dominance of vehicular emissions along with coal (or gas) burning as the key source of ambient PCDD/Fs in the residential areas studied.

KW - Gas/particle partitioning

KW - PCDD/Fs

KW - Residential area

KW - Seasonal variation

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DO - 10.1007/s13762-013-0389-7

M3 - Article

AN - SCOPUS:84919913384

VL - 11

SP - 1897

EP - 1910

JO - International Journal of Environmental Science and Technology

JF - International Journal of Environmental Science and Technology

SN - 1735-1472

IS - 7

ER -

Partitioning of dioxins (PCDDs/Fs) in ambient air at urban residential locations

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Keywords

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