Photocatalytic Efficacy of 1-Dimensional Nanocomposite Electrode

Jung Kun Lee, Bo Ding, Jun Hong Noh, Kug Sun Hong

Research output: Chapter in Book/Report/Conference proceedingChapter

Abstract

The photocatalytic splitting of water into H2 and O2 by oxide nanoparticles has received much attention. However, the full potential of photo-catalysts for efficient hydrogen generation out of water has not been fully realized yet due to unresolved limitations including the low electrical conductivity and ineffective carrier extraction. Here, we report composite oxide materials consisting of 1-dimensional (1-D) transparent conducting oxide (TCO) core and Ti0 2 shell. Highly conductive ITO nanowires were grown on a flexible SUS mesh as a core component. The photoelectrodes consisting of these 1-D nanocomposites have increased carrier mobility due to the TCO core, while the T1O2 shell provides the photocatalytic functionalities. In addition, the built-in-potential at the interface between TCO core and the T1O 2 shell improves the collection of charge carriers from T1O 2 to TCO. These factors altogether contribute to increasing the photocurrent of the device under light.

Original languageEnglish
Title of host publicationEnergy Technology 2012
Subtitle of host publicationCarbon Dioxide Management and Other Technologies
PublisherJohn Wiley and Sons
Pages9-13
Number of pages5
ISBN (Print)9781118291382
DOIs
Publication statusPublished - 2012 May 15
Externally publishedYes

Fingerprint

Oxides
Nanocomposites
Electrodes
Water
Carrier mobility
Charge carriers
Photocurrents
Nanowires
Hydrogen
Nanoparticles
Catalysts
Composite materials

Keywords

  • Core-shell
  • Nanowire
  • Photocatalysis

ASJC Scopus subject areas

  • Materials Science(all)

Cite this

Lee, J. K., Ding, B., Noh, J. H., & Hong, K. S. (2012). Photocatalytic Efficacy of 1-Dimensional Nanocomposite Electrode. In Energy Technology 2012: Carbon Dioxide Management and Other Technologies (pp. 9-13). John Wiley and Sons. https://doi.org/10.1002/9781118365038.ch2

Photocatalytic Efficacy of 1-Dimensional Nanocomposite Electrode. / Lee, Jung Kun; Ding, Bo; Noh, Jun Hong; Hong, Kug Sun.

Energy Technology 2012: Carbon Dioxide Management and Other Technologies. John Wiley and Sons, 2012. p. 9-13.

Research output: Chapter in Book/Report/Conference proceedingChapter

Lee, JK, Ding, B, Noh, JH & Hong, KS 2012, Photocatalytic Efficacy of 1-Dimensional Nanocomposite Electrode. in Energy Technology 2012: Carbon Dioxide Management and Other Technologies. John Wiley and Sons, pp. 9-13. https://doi.org/10.1002/9781118365038.ch2
Lee JK, Ding B, Noh JH, Hong KS. Photocatalytic Efficacy of 1-Dimensional Nanocomposite Electrode. In Energy Technology 2012: Carbon Dioxide Management and Other Technologies. John Wiley and Sons. 2012. p. 9-13 https://doi.org/10.1002/9781118365038.ch2
Lee, Jung Kun ; Ding, Bo ; Noh, Jun Hong ; Hong, Kug Sun. / Photocatalytic Efficacy of 1-Dimensional Nanocomposite Electrode. Energy Technology 2012: Carbon Dioxide Management and Other Technologies. John Wiley and Sons, 2012. pp. 9-13
@inbook{5470d062384c473cbb46d05866dca12e,
title = "Photocatalytic Efficacy of 1-Dimensional Nanocomposite Electrode",
abstract = "The photocatalytic splitting of water into H2 and O2 by oxide nanoparticles has received much attention. However, the full potential of photo-catalysts for efficient hydrogen generation out of water has not been fully realized yet due to unresolved limitations including the low electrical conductivity and ineffective carrier extraction. Here, we report composite oxide materials consisting of 1-dimensional (1-D) transparent conducting oxide (TCO) core and Ti0 2 shell. Highly conductive ITO nanowires were grown on a flexible SUS mesh as a core component. The photoelectrodes consisting of these 1-D nanocomposites have increased carrier mobility due to the TCO core, while the T1O2 shell provides the photocatalytic functionalities. In addition, the built-in-potential at the interface between TCO core and the T1O 2 shell improves the collection of charge carriers from T1O 2 to TCO. These factors altogether contribute to increasing the photocurrent of the device under light.",
keywords = "Core-shell, Nanowire, Photocatalysis",
author = "Lee, {Jung Kun} and Bo Ding and Noh, {Jun Hong} and Hong, {Kug Sun}",
year = "2012",
month = "5",
day = "15",
doi = "10.1002/9781118365038.ch2",
language = "English",
isbn = "9781118291382",
pages = "9--13",
booktitle = "Energy Technology 2012",
publisher = "John Wiley and Sons",

}

TY - CHAP

T1 - Photocatalytic Efficacy of 1-Dimensional Nanocomposite Electrode

AU - Lee, Jung Kun

AU - Ding, Bo

AU - Noh, Jun Hong

AU - Hong, Kug Sun

PY - 2012/5/15

Y1 - 2012/5/15

N2 - The photocatalytic splitting of water into H2 and O2 by oxide nanoparticles has received much attention. However, the full potential of photo-catalysts for efficient hydrogen generation out of water has not been fully realized yet due to unresolved limitations including the low electrical conductivity and ineffective carrier extraction. Here, we report composite oxide materials consisting of 1-dimensional (1-D) transparent conducting oxide (TCO) core and Ti0 2 shell. Highly conductive ITO nanowires were grown on a flexible SUS mesh as a core component. The photoelectrodes consisting of these 1-D nanocomposites have increased carrier mobility due to the TCO core, while the T1O2 shell provides the photocatalytic functionalities. In addition, the built-in-potential at the interface between TCO core and the T1O 2 shell improves the collection of charge carriers from T1O 2 to TCO. These factors altogether contribute to increasing the photocurrent of the device under light.

AB - The photocatalytic splitting of water into H2 and O2 by oxide nanoparticles has received much attention. However, the full potential of photo-catalysts for efficient hydrogen generation out of water has not been fully realized yet due to unresolved limitations including the low electrical conductivity and ineffective carrier extraction. Here, we report composite oxide materials consisting of 1-dimensional (1-D) transparent conducting oxide (TCO) core and Ti0 2 shell. Highly conductive ITO nanowires were grown on a flexible SUS mesh as a core component. The photoelectrodes consisting of these 1-D nanocomposites have increased carrier mobility due to the TCO core, while the T1O2 shell provides the photocatalytic functionalities. In addition, the built-in-potential at the interface between TCO core and the T1O 2 shell improves the collection of charge carriers from T1O 2 to TCO. These factors altogether contribute to increasing the photocurrent of the device under light.

KW - Core-shell

KW - Nanowire

KW - Photocatalysis

UR - http://www.scopus.com/inward/record.url?scp=84886347354&partnerID=8YFLogxK

UR - http://www.scopus.com/inward/citedby.url?scp=84886347354&partnerID=8YFLogxK

U2 - 10.1002/9781118365038.ch2

DO - 10.1002/9781118365038.ch2

M3 - Chapter

AN - SCOPUS:84886347354

SN - 9781118291382

SP - 9

EP - 13

BT - Energy Technology 2012

PB - John Wiley and Sons

ER -