Photon echoes and related four-wave-mixing spectroscopies using phase-locked pulses

Minhaeng Cho; Norbert F. Scherer; Graham R. Fleming; Shaul Mukamel

doi:10.1063/1.462686

Photon echoes and related four-wave-mixing spectroscopies using phase-locked pulses

Minhaeng Cho, Norbert F. Scherer, Graham R. Fleming, Shaul Mukamel

Research output: Contribution to journal › Article › peer-review

126 Citations (Scopus)

Abstract

The use of phase-locked pulses in various spectroscopic techniques related to the third-order polarization P⁽³⁾ is analyzed. Using correlation function expressions for the nonlinear response function, we clarify the interrelationship among several photon echo, pump-probe, and spontaneous light emission techniques, without alluding to any specific model for the material system. By combining phase-locked pulses and heterodyne detection it becomes possible to probe separately the real and imaginary parts of the nonlinear response function. Combining two phase-locked pulse excitation with time-resolved detection of the spontaneous light emission allows direct separation of the Raman and fluorescence contributions.

Original language	English
Pages (from-to)	5618-5629
Number of pages	12
Journal	The Journal of chemical physics
Volume	96
Issue number	8
DOIs	https://doi.org/10.1063/1.462686
Publication status	Published - 1992
Externally published	Yes

ASJC Scopus subject areas

Physics and Astronomy(all)
Physical and Theoretical Chemistry

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title = "Photon echoes and related four-wave-mixing spectroscopies using phase-locked pulses",

abstract = "The use of phase-locked pulses in various spectroscopic techniques related to the third-order polarization P(3) is analyzed. Using correlation function expressions for the nonlinear response function, we clarify the interrelationship among several photon echo, pump-probe, and spontaneous light emission techniques, without alluding to any specific model for the material system. By combining phase-locked pulses and heterodyne detection it becomes possible to probe separately the real and imaginary parts of the nonlinear response function. Combining two phase-locked pulse excitation with time-resolved detection of the spontaneous light emission allows direct separation of the Raman and fluorescence contributions.",

author = "Minhaeng Cho and Scherer, {Norbert F.} and Fleming, {Graham R.} and Shaul Mukamel",

year = "1992",

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journal = "Journal of Chemical Physics",

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T1 - Photon echoes and related four-wave-mixing spectroscopies using phase-locked pulses

AU - Cho, Minhaeng

AU - Scherer, Norbert F.

AU - Fleming, Graham R.

AU - Mukamel, Shaul

PY - 1992

Y1 - 1992

N2 - The use of phase-locked pulses in various spectroscopic techniques related to the third-order polarization P(3) is analyzed. Using correlation function expressions for the nonlinear response function, we clarify the interrelationship among several photon echo, pump-probe, and spontaneous light emission techniques, without alluding to any specific model for the material system. By combining phase-locked pulses and heterodyne detection it becomes possible to probe separately the real and imaginary parts of the nonlinear response function. Combining two phase-locked pulse excitation with time-resolved detection of the spontaneous light emission allows direct separation of the Raman and fluorescence contributions.

AB - The use of phase-locked pulses in various spectroscopic techniques related to the third-order polarization P(3) is analyzed. Using correlation function expressions for the nonlinear response function, we clarify the interrelationship among several photon echo, pump-probe, and spontaneous light emission techniques, without alluding to any specific model for the material system. By combining phase-locked pulses and heterodyne detection it becomes possible to probe separately the real and imaginary parts of the nonlinear response function. Combining two phase-locked pulse excitation with time-resolved detection of the spontaneous light emission allows direct separation of the Raman and fluorescence contributions.

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