TY - JOUR
T1 - Recycling Polymeric Solid Wastes for Energy-Efficient Water Purification, Organic Distillation, and Oil Spill Cleanup
AU - Gong, Feng
AU - Li, Hao
AU - Yuan, Xiangzhou
AU - Huang, Jigang
AU - Xia, Dawei
AU - Papavassiliou, Dimitrios V.
AU - Xiao, Rui
AU - Yamauchi, Yusuke
AU - Wu, Kevin C.W.
AU - Ok, Yong Sik
N1 - Funding Information:
F.G., H.L., and X.Y. contributed equally to this work. The authors would like to acknowledge the financial support of the National Natural Science Foundation of China (52076045, 51525601), the Ministry of Science and Technology of China (2018YFC1902600), and the Ministry of Science and Technology, Taiwan (108‐2638‐E‐002‐003‐MY2 [Shackleton Program award]). F.G. would like to acknowledge the support of “Zhishan Scholar” at Southeast University. This research was supported by the Hydrogen Energy Innovation Technology Development Program of the National Research Foundation of Korea (NRF) funded by the Korean government (Ministry of Science and ICT [MSIT], No. NRF‐2019M3E6A1064197). This work was performed in part at the Australian National Fabrication Facility Queensland Node (ANFF‐Q), a company established under the National Collaborative Research Infrastructure Strategy to provide nano‐ and micro‐fabrication facilities for Australia's researchers.
Funding Information:
F.G., H.L., and X.Y. contributed equally to this work. The authors would like to acknowledge the financial support of the National Natural Science Foundation of China (52076045, 51525601), the Ministry of Science and Technology of China (2018YFC1902600), and the Ministry of Science and Technology, Taiwan (108-2638-E-002-003-MY2 [Shackleton Program award]). F.G. would like to acknowledge the support of ?Zhishan Scholar? at Southeast University. This research was supported by the Hydrogen Energy Innovation Technology Development Program of the National Research Foundation of Korea (NRF) funded by the Korean government (Ministry of Science and ICT [MSIT], No. NRF-2019M3E6A1064197). This work was performed in part at the Australian National Fabrication Facility Queensland Node (ANFF-Q), a company established under the National Collaborative Research Infrastructure Strategy to provide nano- and micro-fabrication facilities for Australia's researchers.
Publisher Copyright:
© 2021 Wiley-VCH GmbH.
PY - 2021/11/18
Y1 - 2021/11/18
N2 - Conventional approaches (e.g., pyrolysis) for managing waste polymer foams typically require highly technical skills and consume large amounts of energy resources. This paper presents an ultrafacile, cost-effective, and highly efficient alternative method for recycling waste packaging and cleaning foam (e.g., polymelamine–formaldehyde foam). The designed solar absorber, a polypyrrole-coated melamine foam (PMF), features a highly porous structure, excellent mechanical strength, low thermal conductivity, and rapid water transport capacity. These exceptional properties render the PMF suitable for multiple applications, including energy-efficient solar-powered water purification, ethanol distillation, and oil absorption. In water purification, the PMF yields a solar–thermal conversion efficiency as high as 87.7%, stability that is maintained for more than 35 operation cycles, and antifouling capabilities (when purifying different water types). In solar distillation, the PMF achieves a concentration increase up to 75 vol% when distilling a 10 vol% ethanol solution. In oil absorption, the PMF offers an oil-absorption capacity of ≈70 g g−1 with only a 7% loss in capacity after 100 absorbing–squeezing cycles. Thus, systems combining solar energy with various waste foams are highly promising as durable, renewable, and portable systems for water purification, organic distillation, and oil absorption, especially in remote regions or emergency situations.
AB - Conventional approaches (e.g., pyrolysis) for managing waste polymer foams typically require highly technical skills and consume large amounts of energy resources. This paper presents an ultrafacile, cost-effective, and highly efficient alternative method for recycling waste packaging and cleaning foam (e.g., polymelamine–formaldehyde foam). The designed solar absorber, a polypyrrole-coated melamine foam (PMF), features a highly porous structure, excellent mechanical strength, low thermal conductivity, and rapid water transport capacity. These exceptional properties render the PMF suitable for multiple applications, including energy-efficient solar-powered water purification, ethanol distillation, and oil absorption. In water purification, the PMF yields a solar–thermal conversion efficiency as high as 87.7%, stability that is maintained for more than 35 operation cycles, and antifouling capabilities (when purifying different water types). In solar distillation, the PMF achieves a concentration increase up to 75 vol% when distilling a 10 vol% ethanol solution. In oil absorption, the PMF offers an oil-absorption capacity of ≈70 g g−1 with only a 7% loss in capacity after 100 absorbing–squeezing cycles. Thus, systems combining solar energy with various waste foams are highly promising as durable, renewable, and portable systems for water purification, organic distillation, and oil absorption, especially in remote regions or emergency situations.
KW - pollution remediation
KW - polymeric waste
KW - recycling
KW - sustainable development
KW - water-energy-waste nexus
UR - http://www.scopus.com/inward/record.url?scp=85115913077&partnerID=8YFLogxK
U2 - 10.1002/smll.202102459
DO - 10.1002/smll.202102459
M3 - Article
C2 - 34590405
AN - SCOPUS:85115913077
SN - 1613-6810
VL - 17
JO - Small
JF - Small
IS - 46
M1 - 2102459
ER -