Robust numerical evaluation of circular dichroism from chiral medium/nanostructure coupled systems using the finite-element method

Seojoo Lee, Ji Hun Kang, Seok Jae Yoo, Q Han Park

Research output: Contribution to journalArticle

4 Citations (Scopus)

Abstract

It has been demonstrated that circular dichroism (CD) signals from chiral molecules can be boosted by plasmonic nanostructures inducing strong local electromagnetic fields. To optimize nanostructures to improve CD enhancement, numerical simulations such as the finite element method (FEM) have been widely adopted. However, FEM calculations for CD have been frequently hampered by unwanted numerical artifacts due to improperly discretizing problem spaces. Here, we introduce a new meshing rule for FEM that provides CD simulations with superior numerical accuracy. We show that unwanted numerical artifacts can be suppressed by implementing the mirror-symmetric mesh configuration that generates identical numerical artifacts in the two-opposite circularly polarized waves, which cancel each other out in the final CD result. By applying our meshing scheme, we demonstrate a nanostructure/chiral molecule coupled system from which the CD signal is significantly enhanced. Since our meshing scheme addresses the previously unresolved issue of discriminating between very small CD signals and numerical errors, it can be directly applied to numerical simulations featuring natural chiral molecules which have intrinsically weak chiroptical responses.

Original languageEnglish
Article number8406
JournalScientific Reports
Volume8
Issue number1
DOIs
Publication statusPublished - 2018 Dec 1

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dichroism
finite element method
evaluation
artifacts
molecules
simulation
mesh
electromagnetic fields
mirrors
augmentation
configurations

ASJC Scopus subject areas

  • General

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Robust numerical evaluation of circular dichroism from chiral medium/nanostructure coupled systems using the finite-element method. / Lee, Seojoo; Kang, Ji Hun; Yoo, Seok Jae; Park, Q Han.

In: Scientific Reports, Vol. 8, No. 1, 8406, 01.12.2018.

Research output: Contribution to journalArticle

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