Self-activated ultrahigh chemosensitivity of oxide thin film nanostructures for transparent sensors

Hi Gyu Moon, Young Soek Shim, Do Hong Kim, Hu Young Jeong, Myoungho Jeong, Joo Young Jung, Seung Min Han, Jong Kyu Kim, Jin Sang Kim, Hyung Ho Park, Jong Heun Lee, Harry L. Tuller, Seok Jin Yoon, Ho Won Jang

Research output: Contribution to journalArticle

73 Citations (Scopus)

Abstract

One of the top design priorities for semiconductor chemical sensors is developing simple, low-cost, sensitive and reliable sensors to be built in handheld devices. However, the need to implement heating elements in sensor devices, and the resulting high power consumption, remains a major obstacle for the realization of miniaturized and integrated chemoresistive thin film sensors based on metal oxides. Here we demonstrate structurally simple but extremely efficient all oxide chemoresistive sensors with ∼90% transmittance at visible wavelengths. Highly effective self-activation in anisotropically self-assembled nanocolumnar tungsten oxide thin films on glass substrate with indium-tin oxide electrodes enables ultrahigh response to nitrogen dioxide and volatile organic compounds with detection limits down to parts per trillion levels and power consumption less than 0.2 microwatts. Beyond the sensing performance, high transparency at visible wavelengths creates opportunities for their use in transparent electronic circuitry and optoelectronic devices with avenues for further functional convergence.

Original languageEnglish
Article number588
JournalScientific Reports
Volume2
DOIs
Publication statusPublished - 2012 Sep 17

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Nanostructures
Oxides
Equipment and Supplies
Nitrogen Dioxide
Volatile Organic Compounds
Semiconductors
Heating
Glass
Limit of Detection
Electrodes
Metals
Costs and Cost Analysis

ASJC Scopus subject areas

  • General

Cite this

Moon, H. G., Shim, Y. S., Kim, D. H., Jeong, H. Y., Jeong, M., Jung, J. Y., ... Jang, H. W. (2012). Self-activated ultrahigh chemosensitivity of oxide thin film nanostructures for transparent sensors. Scientific Reports, 2, [588]. https://doi.org/10.1038/srep00588

Self-activated ultrahigh chemosensitivity of oxide thin film nanostructures for transparent sensors. / Moon, Hi Gyu; Shim, Young Soek; Kim, Do Hong; Jeong, Hu Young; Jeong, Myoungho; Jung, Joo Young; Han, Seung Min; Kim, Jong Kyu; Kim, Jin Sang; Park, Hyung Ho; Lee, Jong Heun; Tuller, Harry L.; Yoon, Seok Jin; Jang, Ho Won.

In: Scientific Reports, Vol. 2, 588, 17.09.2012.

Research output: Contribution to journalArticle

Moon, HG, Shim, YS, Kim, DH, Jeong, HY, Jeong, M, Jung, JY, Han, SM, Kim, JK, Kim, JS, Park, HH, Lee, JH, Tuller, HL, Yoon, SJ & Jang, HW 2012, 'Self-activated ultrahigh chemosensitivity of oxide thin film nanostructures for transparent sensors', Scientific Reports, vol. 2, 588. https://doi.org/10.1038/srep00588
Moon, Hi Gyu ; Shim, Young Soek ; Kim, Do Hong ; Jeong, Hu Young ; Jeong, Myoungho ; Jung, Joo Young ; Han, Seung Min ; Kim, Jong Kyu ; Kim, Jin Sang ; Park, Hyung Ho ; Lee, Jong Heun ; Tuller, Harry L. ; Yoon, Seok Jin ; Jang, Ho Won. / Self-activated ultrahigh chemosensitivity of oxide thin film nanostructures for transparent sensors. In: Scientific Reports. 2012 ; Vol. 2.
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