Two-dimensional vibrational spectroscopy. VII. Investigation of the vibronic and vibrational couplings by using novel triply resonant two-dimensional vibrational spectroscopies

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Abstract

Two-dimensional vibrational spectroscopies utilizing electronically resonant optical probe fields were studied. A proper set of selection rules - new information gained using resonant vibrational spectroscopies and key differences from their analogues utilizing off-resonant optical probe pulses - were studied. Vibrationally resonant infrared field-matter interactions or Raman transitions induced by electronically off-resonant fields were used to create a single vibrational coherence state.

Original languageEnglish
Pages (from-to)7746-7755
Number of pages10
JournalJournal of Chemical Physics
Volume113
Issue number18
DOIs
Publication statusPublished - 2000 Nov 8

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Vibrational spectroscopy
probes
spectroscopy
analogs
Infrared radiation
pulses
interactions

ASJC Scopus subject areas

  • Atomic and Molecular Physics, and Optics

Cite this

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abstract = "Two-dimensional vibrational spectroscopies utilizing electronically resonant optical probe fields were studied. A proper set of selection rules - new information gained using resonant vibrational spectroscopies and key differences from their analogues utilizing off-resonant optical probe pulses - were studied. Vibrationally resonant infrared field-matter interactions or Raman transitions induced by electronically off-resonant fields were used to create a single vibrational coherence state.",
author = "Minhaeng Cho",
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AB - Two-dimensional vibrational spectroscopies utilizing electronically resonant optical probe fields were studied. A proper set of selection rules - new information gained using resonant vibrational spectroscopies and key differences from their analogues utilizing off-resonant optical probe pulses - were studied. Vibrationally resonant infrared field-matter interactions or Raman transitions induced by electronically off-resonant fields were used to create a single vibrational coherence state.

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