Two-dimensional vibrational spectroscopy. VIII. Infrared optical kerr effect and two-color infrared pump-probe measurements

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Abstract

A theoretical study of the infrared optical Kerr effect (IR-OKE) and two-color infrared pump probe spectroscopies was presented. An intense IR pulse to build up large population on a specific intramolecular vibrationally excited state was involved in the method. The femtosecond optical Kerr effect measurement was utilised to detect the time evolution of the nonequilibrium density matrix after a finite mixing time.

Original languageEnglish
Pages (from-to)9982-9992
Number of pages11
JournalJournal of Chemical Physics
Volume114
Issue number22
DOIs
Publication statusPublished - 2001 Jun 8

ASJC Scopus subject areas

  • Physics and Astronomy(all)
  • Physical and Theoretical Chemistry

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