Abstract
A theoretical study of the infrared optical Kerr effect (IR-OKE) and two-color infrared pump probe spectroscopies was presented. An intense IR pulse to build up large population on a specific intramolecular vibrationally excited state was involved in the method. The femtosecond optical Kerr effect measurement was utilised to detect the time evolution of the nonequilibrium density matrix after a finite mixing time.
Original language | English |
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Pages (from-to) | 9982-9992 |
Number of pages | 11 |
Journal | Journal of Chemical Physics |
Volume | 114 |
Issue number | 22 |
DOIs | |
Publication status | Published - 2001 Jun 8 |
ASJC Scopus subject areas
- Physics and Astronomy(all)
- Physical and Theoretical Chemistry